JOURNALOF
Contaminant
Hydrology
ELSEVIER Journal of Contaminant Hydrology 19 (1995) 261-267
Dispersive-diffusive transport of non-sorbed solute
in multicomponent solutions
Qinhong Hu, Mark L. Brusseau *
429 Shantz, Departmentof Soil and WaterScience, University of Arizona, Tucson,AZ 85721, USA
Received 6 December 1994; accepted after revision 14 March 1995
Abstract
The composition of fuels, mixed-solvent wastes and other contaminants that find their way into
the subsurface are frequently chemically complex. The dispersion and diffusion characteristics of
multicomponent solutions in soil have rarely been compared to equivalent single-solute systems.
The purpose of this work was to examine the diffusive and dispersive transport of single- and
multi-component solutions in homogeneous porous media. The miscible displacement technique
was used to investigate the transport behavior of 14C-labelled 2,4-dichlorophenoxyacetic acid
(2,4-D) in two materials for which sorption of 2,4-D was minimal. Comparison of breakthrough
curves collected for 2,4-D in single- and multi-component solutions shows that there is little, if
any, difference in transport behavior over a wide range of pore-water velocities (70, 7, 0.66 and
0.06 cm h-1). Thus, dispersivities measured with a non-sorbing single-solute solution should be
applicable to multicomponent systems.
1. Introduction
The composition of fuels, mixed-solvent wastes, landfill leachate and other contami-
nants that find their way into the subsurface are frequently chemically complex. Thus,
many contaminated sites have multiple contaminants in the aqueous phase. When
multiple components are present in solution, a primary question to be addressed is the
occurrence of antagonistic or synergistic interactions within the system (Brusseau,
1994). As such, it is important to understand the transport dynamics of multicomponent
solutions. The behavior of multicomponent solutions has been widely investigated in
chemical engineering. However, the dispersion and diffusion characteristics of multi-
* Corresponding author.
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