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ISSN 0003-6838, Applied Biochemistry and Microbiology, 2020, Vol. 56, No. 1, pp. 44–50. © Pleiades Publishing, Inc., 2020.
Russian Text © The Author(s), 2020, published in Prikladnaya Biokhimiya i Mikrobiologiya, 2020, Vol. 56, No. 1, pp. 52–59.
The Screening of Refolding Conditions and Obtainment
of the Recombinant Antistaphylococcal Endolysin LysK
CA
in Active Form from E. coli Inclusion Bodies
A. V. Žydziecki
a,
*, S. G. Golenchenko
a
, U. A. Prakulevich
a
, and M. V. Sholukh
a
a
Belarusian State University, Biology Department, Minsk, 220030 Belarus
*e-mail: Zhydzetski@gmail.com
Received April 17, 2019; revised July 29, 2019; accepted August 30, 2019
Abstract—Step-by-step screening of the main characteristics of refolding buffer is proposed to obtain recom-
binant antistaphylococcal endolysin LysK containing two catalytic domains, CHAP and amidase-2, in active
form from E. coli inclusion bodies. The optimal pH, temperature, redox potential of the refolding buffer, as
well as the optimal protein concentration and type of antiaggregation compound were determined. The compo-
sition of a renaturation system of antistaphylococcal endolysin containing 20 mM phosphate buffer, pH 7.4,
0.4 M sucrose, and 2.5 mM DTT at 10°C with dilution to a final concentration of ~150 μg/mL was found to
be optimal. The refolding yield after scaling was about 29.5 ± 6.7%, which produced 16 ± 2.3 mg of the target
protein from 2.25 g of washed inclusion bodies with a specific enzyme activity of 1.8 ± 0.73 × 10
3
U/mg.
Keywords: recombinant endolysin LysK
CA
, protein refolding, inclusion bodies, screening of renaturation con-
ditions
DOI: 10.1134/S0003683820010160
INTRODUCTION
The technology of recombinant DNA molecules
has opened a new era in the production of various
kinds of proteins, both for structural and biochemical
studies and for industrial and commercial purposes [1].
Expression in transformed cells makes it possible to
obtain rare, valuable, expensive proteins that are diffi-
cult to obtain by traditional methods [2, 3]. In partic-
ular, a number of therapeutic proteins that have great
potential for use in medicine and veterinary medicine
to replace standard treatment methods can be obtained
with this method [4, 5].
One of these proteins is endolysin of phage K (LysK),
a peptidoglycan hydrolase involved in the lysis of
gram-positive bacterial cells of the Staphylococcus
genus that is expressed in the terminal cycle of the
release of mature phage particles from host cells [6–8].
The endolysin LysK consists of three domains, two
catalytic domains (CHAP and amidase-2) and one
structural (SH3b); truncated variants of this protein
containing the CHAP domain also possess activity [9,
10]. The high antistaphylococcal effectiveness of LysK
and its derivatives towards the Staphylococcus genus
makes it a promising candidate as a new antimicrobial
agent in medicine and veterinary medicine, especially
with respect to antibiotic resistant strains. It should be
noted that this protein has several advantages over
standard antistaphylococcal drugs. The main advan-
tages are the lack of the development of resistance, the
manifestation of high species specificity, the absence
of effects on normal microflora, and the safety of its
use in the food industry [8, 11]. However, certain dif-
ficulties in the study and further use of LysK and its
forms are associated with their isolation in limited
quantities. The research on this protein is based in
most cases on its preparation in producer strains in
soluble form with further purification on affinity sor-
bents [7, 8, 12, 13]. However, with this technology, it
is possible to obtain a small amount of protein for
research purposes. In particular, recent studies
obtained only 2–10 mg of CHAP
K
and about 12 mg of
LysK
CA
from 1 L of fermentable culture [13–15]. At
the same time, the potential applications in veterinary
medicine, medicine, and other sectors of the national
economy will require large quantities and, accord-
ingly, cheaper and more effective methods for the pro-
tein production [11]. A sufficient amount of the target
protein can be prepared from inclusion bodies (IBs),
dense, highly hydrated formations consisting mostly
of inactive, aggregated molecules of the target pro-
tein [16]. Although a number of additional difficulties
arise in this case, the main issue is the activation of the
target protein molecules associated with the refolding
process. The effectiveness of the renaturation of
recombinant proteins depends on the competition
between the correct folding and aggregation [17, 18].
The dominant process is determined by the composi-