Science and Engineering Applications 2(3) (2017) 148-151 ISSN-2456-2793(Online)
©Payam Publishing Pvt. Lt. India http://www.jfips.com/ 148
Role of C ion implantation on structural and optical properties
of CeO2 thin films deposited on quartz substrates
Pawan Kumar
1
, Zubida Habib
2*
and Dar Manzoor
3
1
Department of Physics, Kurukshetra University Kurukshetra, Haryana – 136119, India
2
Department of Chemistry, National Institute of Technology, Hazratbal, Srinagar 190006, India
3
Physical Chemistry Division, NCL Pune-411008, India
*Email : zubida.habib@gmail.com
Abstract
This investigation reports on effect of C ion implantation on structure and optical properties of CeO2 thin films deposited on
quartz substrates by the radio frequency (RF)-sputtering method. X-ray diffraction analysis shows that the face-centered cubic
(FCC) structure corresponds to CeO2. The lattice parameter of C ion implanted CeO2 films was found to decrease compared to
that of the pristine CeO2 film. The shift in the peak positions after C ion implantation indicates changed lattice parameters. The
observed values of strain are found to be positive and decreasing value of strain after C ion implantation indicates tensile strain
in all of the prepared CeO2 films. The Raman spectra further confirm the formation of phase and also indicate the presence of
defects in these films. The F2g peak intensity is decreasing with C ion fluence compared with that of the pristine film which is
due to defects created after C ion implantation. Uv-Vis spectra shows that energy band gap decreases with C ion implantation
which indicates increase in conductivity with C ion implantation in the films.
Keywords: CeO2, Ion implantation, Band gap.
DOI: http://dx.doi.org/10.26705.xxx.xxx.xxxx
Received : 17/11/2017 Published online : 25/11/2017
1. Introduction
Ceria based metal oxide materials have several
technological applications and has been extensively studied
[1-5]. These materials are important because of their potential
applications such as UV absorbents and filters, electronic
ceramic, ultra-precise polishing, gas sensor, catalysts and
electrolyte in the fuel cell technology [6], catalytic wet
oxidation, engine exhaust catalysts and photocatalytic
oxidation of water. Most recently, CeO2 nanoparticles have
been tested for their ability to serve as free-radical scavengers
[7-8]. Therefore, the extensive synthesis and study of CeO2
becomes an urgent task for further research and applications
[9-10]. Cerium oxide (CeO2) shows good optical properties
and is a semiconductor with wide band gap energy (3.19eV).
The material’s modification with energetic ion beams shows
interesting technological applications. There are two modes of
materials modification by energetic ion beams, ion
implantation and swift heavy ion (SHI) irradiation. In both of
the techniques, the energy and fluence of incident ions play
an important role [11]. In the ion implantation process, the
energetic ions have low energy (a few tens of keV to a few
hundreds of keV). The desired ions can be implanted in the
suitable material by choosing the various implantation
parameters like type of ion, ion energy, range of ion and ion
fluence etc. and the materials properties get modified due to
the presence of implanted ions. There are several reports
available on the formation of embedded nano phases of target
ions and and effects of such nano phases on the various
properties of host material [12-13]. In this context we have
performed ion implantation experiment with different
fluencies on CeO2 thin films.
Considering the importance of these materials, present study
focuses on understanding of structural and optical properties
of C ion implanted CeO2 thin films deposited by RF
sputtering.
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