STAINLESS AND ELECTRICAL STEELS
UDC 669.14.018.8
HIGH-STRENGTH AUSTENITIC STAINLESS STEEL
V. G. Gavrilyuk
1
and H. Berns
2
Translated from Metallovedenie i Termicheskaya Obrabotka Metallov , No. 12, pp. 17 – 19, December, 2007.
Based on the studies of carbon and nitrogen effects on the electron structure, short-range atomic order, and
thermodynamic stability of iron solid solutions, a physical concept for alloying steels with carbon and nitro-
gen is proposed. The concept is used for the design of a cost-effective austenitic corrosion-resistant steel of
super-high strength and fracture toughness.
INTRODUCTION
Preliminary calculations of electron structure give evi-
dence that the replacement of carbon by nitrogen in g iron in-
creases the density of electron states at the Fermi level, i.e.,
enhances the metallic character of interatomic bonds (see
e.g. [1]). This conclusion is consistent with data on the con-
centration of conduction electrons obtained by measure-
ments of electron spin resonance [1 – 3]. A correlation be-
tween electron structure and short-range atomic order was
shown in [1] where the thermodynamic stability of iron-
based solid solutions is discussed in terms of ordering result-
ing from prevailing metallic interatomic bonds or from clus-
tering caused by covalent bonds.
Subsequent measurements on austenitic steels, where a
part of nitrogen was replaced by carbon, revealed a further
enhancement of the metallic interatomic bonds [4, 5].
These results made it possible to propose a physical con-
cept for alloying steels with carbon together with nitrogen
[4]. The aim of the present study is to show how this concept
can be used for the development of a new austenitic high-
strength corrosion-resistant steel.
RESULTS AND DISCUSSION
Atomic Interactions and Thermodynamics
The concentration of conduction electrons r
c
in
austenitic steels as a function of the C, N or C + N contents is
presented in Fig. 1. Carbon does not cause any significant
change in r
c
, which suggests that it contributes its electrons
to states below the Fermi level, i.e., assists strengthening of
covalent interatomic bonds. With nitrogen content increasing
up to some optimal value of about 0.6 wt.%, r
c
increases and
then decreases at higher nitrogen contents. A remarkable in-
crease of r
c
occurs if some part of nitrogen is replaced by
carbon and, moreover, the maximum of r
c
is shifted to higher
contents of interstitial atoms.
Two conclusions follow from these results: (1 ) the en-
hancement of the metallic character of interatomic bonds due
to alloying with C + N should improve the toughness of
austenitic steels; (2 ) the shift of the r
c
maximum in C + N
Metal Science and Heat Treatment Vol. 49, Nos. 11 – 12, 2007
566
0026-0673/07/1112-0566 © 2007 Springer Science + Business Media, Inc.
1
G. V. Kurdyumov Institute for Metal Physics, Kiev, Ukraine.
2
Ruhr University Bochum, Bochum, Germany.
4.0
3.0
2.0
1.0
0 1.0 2.0 3.0 4.0
0 0.2 0.4 0.6 0.8 1.0 1.2
C(N), wt.%
(Ñ + N), at.%
r
s
– 22
–3
10
, ñm
´
0.5
0.7N
0.88N
0.8
0.95
1.07
Ñ+N
Ñ+N
Fig. 1. Concentration of conduction electrons r
c
in austenitic steels
as a function of C, N or C + N contents: :) Cr13Mn18C0.4N0.4;
=) Cr13Mn18C0.25N0.25; O) Cr19Mn19C0.49N0.58;
N) Cr18Mn19C0.34N0.61; &) Cr18Mn20N0.88; q) Cr13Mn18N0.7;
p) Cr15Mn17N0.45; )) Cr18Ni16Mn10N; ^) Cr18Ni16Mn10C.