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*Corresponding author.
Email: zuraidaa@iium.edu.my
International Food Research Journal 19(2): 715-719 (2012)
*
Zuraida, A., Yusliza, Y., Anuar, H. and Mohd Khairul Muhaimin, R.
Kulliyyah of Engineering, International Islamic University Malaysia, P.O. Box 10,
50728, Kuala Lumpur, Malaysia
The effect of water and citric acid on sago starch bio-plastics
Abstract: Starch is a biodegradable polymer produced in abundance from many renewable resources. This
study examined the infuence of citric acid (0-40% w/wt%) ) and water (0-40% w/wt%) as secondary additive
and glycerol as plasticizer on the mechanical properties of bio-plastic starch (BPS) from Malaysian sago. The
CA content varies from 0 to 40 w/wt% while water was also varied from 0 to 40 w/wt%. FT-IR spectroscopy
showed that acid citric improve the properties of BPS and water give negative effects to the carbon hydrogen-
bond. It is obvious that the addition of the CA at 30 wt/wt% improve the mechanical property of BPS to more
than 40% compare to the addition of water.
Keywords: Component, sago, starch, melt processing, citric acid
Introduction
Particular attention has been given in the recent
years for the development of biodegradable polymers
from renewable resources, especially for packaging
and disposable applications to maintain sustainable
development of economically and ecologically
attractive technology, towards greener environment
(Schlemmer et al., 2010; Fischer et al., 2011). Among
these biopolymer, starch is one of the promising
materials because of its large availability, low cost,
renewable resources and inherent biodegradability
(Shi et al., 2007).
Native starch is the major sources of
polysaccharide in plants. Previously many
researchers have focused on starches from
corn, wheat and potato and very few reports are
available on sago starch. Sago starch is produced
from sago palm (Metroxylon spp.), which is also
known as rumbia. Sago is initially presents in
South East Asia and can be found especially in
Sarawak, Malaysia. Sago starch is commonly
used as functional ingredient (e.g. thickener,
stabilizer, gelling agent) in the food industry
(Mohamed et al., 2008). In order to adjust the
properties of these starch-based materials for
non-edible applications, it requires combination
with other polymers that may need for starch
modifcations such as esterifcation, grafting and
reactive or melting extrusion of thermoplastic
starch (TPS), which is also known as bioplastic
starch (BPS) (Carvalho, 2008).
BPS is an amorphous or semi-crystalline polymeric
material composed of gelatinized or destructurized
starch containing one or a mixture of plasticizer
(Liu et al., 2009). Various plasticizer and additives
have been evaluated for the gelatinization of starch
during thermal processing. Among the plasticizers,
water is the most commonly used in the thermal
processing of starch based polymers. BPS containing
only water alone however, results in poor mechanical
properties such as the brittleness due to the fast
retrogradation (recrystallization). Therefore, other
non-volatile plasticizers are investigated to improve
the processing ability and product properties of the
BPS such as, glycerol, glycol and sorbitol, sugars,
urea, formamide, acetamide,ethylenebisformamide,
ethanolamine and citric acid.
This study was carried out to investigate the
potential of sago starch as natural sources for the
production of BPS and to optimize the process
condition of the starch plasticized with glycerol, and
the effect of water and citric acid as co-plasticizer on
the mechanical and thermal properties of the BPS.
Further, morphological structure of the samples was
observed by using scanning electron microscope
(SEM).
Materials and methods
Materials
Sago starch powder (25% amylose) was purchased
from Hup Seng Heng Sdn Bhd, Malaysia, glycerol
(95% purity) with density of about 1.261 g/cm³ and
citric acid were supplied by Merck.
Fabrication process
In this experiment there were two compositions
prepared. First is a mixture of starch and glycerol.