Research Article Open Access
Mabrouk et al., Bioceram Dev Appl 2013, S:1
DOI: 10.4172/2090-5025.S1-009
ISSN: 2090-5025 BDA, an open access journal Bioceram Dev Appl Conferences Proceedings: ISACB-6
Keywords: Tissue engineering; Scafolds; Ciprofoxacin; Drug
release; Freeze drying; Polyvinyl alcohol
Introduction
Bioactive glass (BG) has various applications in repair and
reconstruction of bone tissue; however, it has week mechanical
properties especially in porous form. One approach to enhance
the mechanical properties of materials is the elaboration of BG
with polymer to form composites [1]. Tis way leads to an excellent
combination between strength and toughness, as well as improved
characteristics, when compared to their individual components [2].
Te composites of BG/polymer are able to provide construct with
excellent osteogensis and angiogenesis [1]. Application of a drug to a
specifc region using drug loaded scafold produce high concentration
of the drug in the required site of action which eliminate the side efects
that prohibit the administration of large oral dose. Ciprofoxacin (Cip)
is a furoquinolone derivative, widely used as an antibiotic and in
osteomyelitis because of its favorable penetration and bactericidal efect
on all the probable osteomyelitis pathogens [3]. Te main purpose of
the current study was to develop and fabricate a construct of bioactive
scafold combining an antibiotic (ciprofoxacin) as a target drug delivery
system. Characterization of these scafolds before and afer addition of
the drug has been investigated by XRD, FTIR, mercury porosimeter,
SEM, universal testing machine and UV-spectrophotometer.
Materials and Methods
Synthesis
Te 46S6 bioactive glass was prepared as previously reported [4]
by using calcium silicate (Alfa Aesar), trisodium trimeta phosphate
and sodium metasilicate pentahydrate (Sigma). Te prepared glass was
named MB. Polyvinyl alcohol (PVA) and polyvinyl alcohol/bioactive
glass in molar ratio 1:2 PVA/MB scafolds and scafolds loaded with
ciprofoxacin drug (PVA/MB-cip) were prepared by employing
thermally induced phase separation technique (freeze drying). Firstly,
15% of PVA (Aldrich, M. wt= 67.000) was dissolved in distilled water
at 80°C for 2 hr. Te prepared glass MB was added to polymer solution
with continuous stirring at room temperature for 20 hr. Ten, exactly
5, 10 and 20% of ciprofoxacin drug were added to the batch of PVA
and to that of PVA/MB composite with stirring for 1 hr. Afer that, the
mixture was poured in moulds to form cylinders with diameters of 15
mm × 10 mm and kept at -18°C overnight, then transferred to a freeze
dryer type Christ, Alpha 1-2 LD plus for 24 hr.
Characterizations
Te porosity and the micro architecture of the prepared scafolds
were assessed by means of Mercury Intrusion Porosimetry (MIP) by
using Poresizer 9320 V2.08, liquid displacement method and scanning
electron microscopy (SEM) (Jeol JSM 6301).Te phases and structure
of each components of the prepared scafold had been examined by
XRD (Philips X-PERT with Cu Kα wave length of 1.5418 Å) and
FTIR (Nicolet Magna-IR 550). Compressive strength was measured
by universal testing machine type Lloyd. Te release of the drug was
constructed in PBS at pH 7.4 and drug concentration was followed
using UV-spectrophotometer (Jenway 6705) at 277 nm.
Results and Discussion
Morphological and microstructural properties
Te morphology of the prepared scafolds is presented in (Figure
*Corresponding author: AA Mostafa, University of Rennes 1, UMR CNRS
6226, 263 av. du général leclerc, 35042 Rennes Cedex, France, E-mail:
amany.mostafa@univ-rennes1.fr
Received May 13, 2013; Accepted May 30, 2013; Published September 10, 2013
Citation: Mabrouk M, Mostafa AA, Oudadesse H, Mahmoud AA, Gaafar AM, et al.
(2013) Fabrication, Characterization and Drug Release of Ciprofoxacin Loaded
Porous Polyvinyl Alcohol/Bioactive Glass Scaffold for Controlled Drug Delivery.
Bioceram Dev Appl S1: 009. doi: 10.4172/2090-5025.S1-009
Copyright: © 2013 Mabrouk M, et al. This is an open-access article distributed
under the terms of the Creative Commons Attribution License, which permits
unrestricted use, distribution, and reproduction in any medium, provided the
original author and source are credited.
Abstract
Composite scaffolds of polyvinyl alcohol (PVA) and/or quaternary bioactive glass (46S6 system) containing 5, 10 and
20 wt % ciprofoxacin were prepared by lyophilisation technique. The porosity of the prepared scaffolds was measured
by liquid displacement, Hg-porosimeter and SEM. The structure and the nature of chemical bonds between atoms were
examined by XRD and FTIR. They confrmed the incorporation of ciprofoxacin into the scaffolds. Biodegradation rate
and drug release behaviour were conducted in phosphate buffer saline (PBS) at pH 7.4. A porous scaffold has been
obtained with porosity up to 85%. By increasing the glass contents and drug concentration in the prepared scaffold the
porosity and the degradation rate decrease however, the compressive strength was enhanced. A sustained drug release
pattern was observed from the optimized scaffold with a quasi-Fickian diffusion mechanism and it was able to deliver
the drug in a prolonged release pattern which offers a distinguish treatment for osteomylitis as well as local antibacterial
effect.
Fabrication, Characterization and Drug Release of Ciprofloxacin Loaded
Porous Polyvinyl Alcohol/Bioactive Glass Scaffold for Controlled Drug
Delivery
M Mabrouk
1,2
, AA Mostafa
1,2
*, H Oudadesse
1
, AA Mahmoud
3
, AM Gaafar
4
and MI El-Gohary
5
1
University of Rennes 1, UMR CNRS 6226, 263 av. du général leclerc, 35042 Rennes Cedex, France
2
Biomaterials Department, National Research Centre, Cairo, Egypt
3
Pharmaceutical Technology National Research Centre (NRC), Cairo, Egypt
4
Photo Chemistry Department, National Research Centre (NRC), Cairo, Egypt
5
Physics Department, Faculty of Science, Al -Azhar University, Cairo, Egypt
Bioceramics Development
and Applications
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ISSN: 2090-5025