Proceedings of International Structural Engineering and Construction, 9(1), 2022
State-of-the-art Materials and Techniques in Structural Engineering and Construction
Edited by Holschemacher, K., Quapp, U., Singh, A., and Yazdani, S.
Copyright © 2022 ISEC Press
ISSN: 2644-108X
www.doi.org/10.14455/ISEC.2022.9(1).AAC-10
AAC-10-1
THE EFFECT OF RE-CALCINATION FLY ASH ON
GEOPOLYMER PERFORMANCE
M SHAHIB AL BARI
1
, JANUARTI JAYA EKAPUTRI
1
, RASGIANTI
2
, BERNARDED OKA
ANGGARANI
2
, and PRASETYO ADI WIBOWO
2
1
Dept of Civil Engineering, Institut Teknologi Sepuluh Nopember, Surabaya, Indonesia
2
PT PLN (Persero) Research Institute, South Jakarta, Indonesia
Geopolymer is one of the concrete technologies to utilize fly ash from coal combustion
residue. However, the unburnt carbon in fly ash deteriorates the mechanical properties.
To reduce the carbon, the calcination is required. This study presents the effect of
calcination at 1000
o
C on five samples of fly ash. All fly ashes were activated with alkali
activator having a mass ratio of Na2SiO3 to NaOH was kept constant at 2. Compression
test was conducted at 3, 7, 14, 21, 28, and 56 days to obtain the effect of calcination to
the compressive strength. It was found that the Si/Al ratio significantly affected the
compression strength. The calcination reduced the carbon content in fly ash. However,
amorphous phase of fly ash dropped after calcination as all the compression test result
were less than 1 MPa. the calcination hindered the geopolymerization as all of the setting
time exceeded seven days causing no compressive strength at early age.
Keywords: Cementitious materials, Alkali activated materials, Si/Al, Soluble silica.
1 INTRODUCTION
Fly ash is one of coal combustion residues that has been used in many sectors, mainly in
construction and materials. However, only low loss of ignition (LOI) fly ash is accepted by cement
producers following ASTM C618-19. LOI is the sum of burnable organic components, which
contains mainly carbon. However, the LOI does not provide the form and properties of carbon
which remained mystery on its effect on concrete (Freeman et al. 1997). Carbon has three effects
on concrete: discoloration, lowering air entrainment behavior, and corrosion resistance (Freeman
et al. 1997, Ha et al. 2005). High carbon of fly ash tends to have black color which is not preferable.
Meanwhile, higher carbon content adsorbs more water and chemical content, such as
superplasticizer and air entrainment agent (AEA) which decreases the workability and reduce
freeze-thaw resistance (Freeman et al. 1997, Pedersen et al. 2008). The corrosion rate of rebar also
increases when the LOI in fly ash is more than 6% (Ha et al. 2005). It is important to understand
the effect of LOI and its removal using sintering method.
LOI affects not only on Portland concrete, but also on geopolymer. High LOI in fly ash lowers
compressive strength of geopolymer (Nurwidayati et al. 2016). To reduce LOI content, Temuujin
and Riessen (2009) burned fly ash at 500
o
C and 800
o
C. It was found that the geopolymer
performance was reduced which was caused by change of amorphous phase and crystallization on
the surface of particles.
This paper discusses the effect of calcination at 1000
o
C on five high-carbon fly ashes from
circulating fludizied bed combustion (CFBC) boilers which their steam temperature is under 850
o
C. Due to the low combustion temperature, CFBC fly ash has low reactivity and irregular shape