Advances in Chemical Engineering and Science, 2011, 1, 245-251
doi:10.4236/aces.2011.14035 Published Online October 2011 (http://www.SciRP.org/journal/aces)
Copyright © 2011 SciRes. ACES
Pretreatment of Wastewater Streams from
Petroleum/Petrochemical Industries Using Coagulation
Hossam Altaher
*
, Emad ElQada, Waid Omar
Chemical Engineering Technology Department, Yanbu Industrial College, Saudi Arabia
E-mail:
*
haltaher@hotmail.com (or haltaher@vt.edu)
Received June 27, 2011; revised July 19, 2011; accepted August 12, 2011
Abstract
Coagulation-flocculation processes using different types of conventional coagulants, namely, ferric chloride
(FeCl
3
), aluminum sulfate (AL
2
(SO4)
3
·18H
2
O), lime and ferrous sulfate (FeSO
4
) were investigated using the
Jar-test technique. A further aim is to determine the optimum conditions for the treatment of industrial
wastewater effluents i.e. coagulant dosage, mixing rate, temperature and pH control. Under optimal condi-
tion of process parameters, coagulation/flocculation process was able to lower the turbidity well below the
permissible level (1.8 NTU). The results indicate that ferric chloride had superior efficiency compared with
other coagulants with efficient dose of 800 mg/l. The optimal initial pH of the effluents that enhanced the
turbidity removal was 8.6. The temperature showed no significant effect on the turbidity removal.
Keywords: Ferric Chloride, Coagulation, Wastewater, Petrochemicals, Pretreatment
1. Introduction
This template, Yanbu Industrial City, at the Red Sea
Coast of Saudi Arabia, is considered as one of the major
industrial cities in the Kingdom of Saudi Arabia. The
city accommodates several large refining and petro-
chemical plants as well as a broad range of other manu-
facturing and support enterprises [1]. This inexorable
growth in the scale of the petrochemical industries and
oil refinery was largely responsible for the remarkable
ecological problems at Yanbu Industrial City.
This forces the Saudi government to issue strict legis-
lation concerning the quality of industrial wastewater
effluents and the industries are not allowed to discharge
any treated or untreated effluent in open channels and
even after treatment, the reclaimed water must have to
comply with direct discharge standards before discharge
to the sea [2]. So the entire industrial sectors send their
wastewater effluents to a local wastewater treatment
plant to treat their waste effluents to an increasingly high
standard. Actually, the treatment system consisting of
physical, chemical, and biological units is not enough in
its current state to reach the permissible levels of dis-
charge especially for turbidity. However, the focus of
this paper is the enhancement of coagulation process in
an attempt to comply with turbidity standards for obvi-
ous health issues.
Coagulation, adsorption on activated carbon, precipi-
tation, evaporation, ion-exchange, oxidation, and bio-
degradation and membrane filtration are known as an
industrial pollution prevention technology and used for
the decontamination of contaminated water and waste-
water [3]. According to Renault et al. [3], complete
treatment will clearly require several steps and it is often
appropriate to combine several methods of purification
before maximal efficiency is obtained.
Coagulation/flocculation is a widely-used process in
the primary purification of water and in industrial
wastewater treatment [3-5]. This method has a prefer-
ence in the primary purification processes mainly due to
the ease of operation, high efficiency, cost effective Also,
it uses less energy than alternative treatment [5-7].
Coagulants, both inorganic and organic such as alu-
minum sulfate (alum), ferrous sulfate, ferric chloride and
ferric chloro-sulfate are widely used as coagulants in
water and wastewater treatment for removing a broad
range of impurities from effluent, including organic mat-
ter, turbidity, color, microorganism, colloidal particles
and dissolved organic substances [4,5,8-10]
Wang et al [11] demonstrated that many factors can
influence the efficiency of coagulation-flocculation pro-
cess such as the type and dosage of coagulant/floccu-
lant, pH, mixing speed and time, temperature and reten-
tion time. An appropriate combination of these factors is