Vol.:(0123456789) 1 3
Journal of Radioanalytical and Nuclear Chemistry
https://doi.org/10.1007/s10967-018-6310-6
Sorption of Am(III) on clays and clay minerals: A review
Daniel R. Fröhlich
1
· Ugras Kaplan
2
Received: 13 August 2018
© Akadémiai Kiadó, Budapest, Hungary 2018
Abstract
The problem connected to the long-term storage of high-level nuclear waste has initiated an extensive search for suitable
host rock formations and backfll materials to guarantee an isolation of hazardous nuclear elements from the biosphere
for thousands of years. Besides other alternatives, clays and clayey materials have been in the focus of various sorption
studies. With respect to long-term predictions of migration processes, the transuranium elements and fssion products
are of particular interest. The present review gives a detailed summary of sorption studies conducted during the past
decades describing the impact of various geochemical parameters on the immobilization of Am(III) by diferent clays
and clay minerals.
Keywords Americium · Sorption · Clay minerals · Nuclear waste disposal
Introduction
The search for suitable host rock formations for the fnal
disposal of high-level nuclear waste has lead to strong
scientifc efort worldwide with the aim of weighing the
advantages and disadvantages of diferent potential host
rocks. Besides rock salt and crystalline formations (e.g.
granite), clay rocks are considered and investigated in
various countries (e.g. Belgium [ 1], China [ 2], France
[3], Germany [4], and Switzerland [5]). Furthermore, the
potential backfll material bentonite, which is considered
in various nuclear waste repository scenarios, is mainly
constituted of clay (typically 60–80% montmorillonite)
as well.
Positive characteristics of clays include a high sorption
capacity for heavy metals and the self-healing of cracks
due to swelling. Therefore, a strong retardation of radio-
nuclides, when released from their primary containment
during storage, is assumed. With respect to long-term pre-
dictions and any safety assessment, the long-lived radio-
nuclides, which will determine the long-term radiotoxicity
of the waste material, are of particular interest. These
include the transuranium elements Np, Pu and Am, whose
geochemistry and migration behavior is thus of high
importance.
The relevant geochemical processes include sorption onto
and difusion in the clay, complexation reactions with poten-
tial ligands in the deep waters, and dissolution/precipitation
reactions. All of these processes are strongly dependent on
the characteristic geochemical conditions of the potential
storage site. Important parameters include pH, redox poten-
tial, ionic strength, temperature and inorganic (especially
carbonate) or organic ligands (e.g. humic substances) which
are ubiquitous found in natural waters.
Due to the strongly reducing conditions expected in the
near-feld of a nuclear waste repository, resulting from the
corrosion of the steel containments, + 3 (Pu, Am) and + 4
(Np) will be the predominant oxidation states of the tran-
suranium elements [6]. Therefore, various studies during
the past decades have focused on the interaction between
trivalent actinides with clays. Compared to Pu(III), Am(III)
ofers a strong advantage through its redox stability, which
simplifes the chemical handling.
Diferent modeling approaches to describe the uptake
mechanisms of actinides by various sorbents, including
clays, have been the topic of a very extensive review by
Geckeis et al. [7]. The present work is a continuation of the
* Daniel R. Fröhlich
daniel.froehlich@partner.kit.edu
1
Institute of Physical Chemistry, Ruprecht-Karls-University
Heidelberg, Im Neuenheimer Feld 253, 69120 Heidelberg,
Germany
2
Karlsruhe, Germany