Open Journal of Physical Chemistry, 2021, 11, 13-53
https://www.scirp.org/journal/ojpc
ISSN Online: 2162-1977
ISSN Print: 2162-1969
DOI: 10.4236/ojpc.2021.112002 Mar. 25, 2021 13 Open Journal of Physical Chemistry
Heat Capacity and Bond Dissociation Energy
Calculations of Some Fluorinated Ethanol’s and
its Radicals: CH
3−x
CH
2
F
x
OH, CH
3
CH
2−x
F
x
OH
Hebah M. Abdel-Wahab, Joseph W. Bozzelli
Department of Chemistry and Environmental Science, New Jersey Institute of Technology, Newark, New Jersey, USA
Abstract
Structures and thermochemical properties of these species were determined
by the gaussian M-062x/6-31 + g (d, p) calculation enthalpies of formation
for 19 fluorinated ethanol and some radicals were calculated with a popular
Ab initio and density functional theory methods: The gaussian M-062x/6-31
+ g (d, p) via several series of isodesmic reactions. Entropies (S298˚K in
Cal∙Mol
−1
K
−1
) were estimated using the M-062x/6-31 + g (d, p) computed
frequencies and geometries. Contributions of entropy, S298˚K, and heat ca-
pacities, Cp(T) due to vibration, translation, and external rotation of the mo-
lecules were calculated based on the vibration frequencies and structures ob-
tained from the M-062x/6-31 + g (d, p) Density Functional Method. Potential
barriers are calculated using M-062x/6-31 + g (d, p) density functional me-
thod and are used to calculate rotor contributions to entropy and heat capac-
ity using integration over energy levels of rotational potential. Rotational bar-
riers were determined and hindered internal rotational contributions for
S298˚ - 1500˚K, and Cp (T) were calculated using the rigid rotor harmonic
oscillator approximation, with direct integration over energy levels of the
intramolecular rotation potential energy curves. Thermochemical properties
of fluorinated alcohols are needed for understanding their stability and reac-
tions in the environment and in thermal processes.
Keywords
Thermo-Chemistry, Enthalpy, Fluorinated Ethanol’s, Thermochemical Properties
1. Introduction
Fluorinated hydrocarbons are used as refrigerants, in polymers, heat exchange
fluids, and as solvents. They are present in the atmosphere, lithosphere, and hy-
How to cite this paper: Abdel-Wahab,
H.M. and Bozzelli, J.W. (2021) Heat Ca-
pacity and Bond Dissociation Energy Cal-
culations of Some Fluorinated Ethanol’s and
its Radicals: CH
3−x
CH
2
F
x
OH, CH
3
CH
2−x
F
x
OH.
Open Journal of Physical Chemistry, 11,
13-53.
https://doi.org/10.4236/ojpc.2021.112002
Received: October 26, 2020
Accepted: March 22, 2021
Published: March 25, 2021
Copyright © 2021 by author(s) and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access