Research Article
An Autopsy of Nanofiltration Membrane Used for
Landfill Leachate Treatment
Ibrahim Demir,
1
Ismail Koyuncu,
1,2
Serkan Guclu,
1,2
Senol Yildiz,
3
Vahit Balahorli,
3
Suphi Caglar,
3
Turker Turken,
1,2
Mehmet E. Pasaoglu,
1,2
Recep Kaya,
1,2
and Reyhan Sengur-Tasdemir
2,4
1
Environmental Engineering Department, Istanbul Technical University, Maslak, 34469 Istanbul, Turkey
2
National Research Center on Membrane Technologies (MEM-TEK), Istanbul Technical University, Maslak, 34469 Istanbul, Turkey
3
ISTAC, Istanbul Environmental Management in Industry and Trade Inc., 34379 Istanbul, Turkey
4
Nanoscience and Nanoengineering Department, Istanbul Technical University, Maslak, 34469 Istanbul, Turkey
Correspondence should be addressed to Ibrahim Demir; idemir@itu.edu.tr
Received 24 February 2015; Accepted 13 May 2015
Academic Editor: Ghadir A. El-Chaghaby
Copyright © 2015 Ibrahim Demir et al. Tis is an open access article distributed under the Creative Commons Attribution License,
which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
Komurcuoda leachate treatment plant, Istanbul, which consists of membrane bioreactor (MBR) and nanofltration (NF) system,
faced rapid fux decline in membranes afer 3-year successful operation. To compensate rapid fux decline in membranes, the
fouled membranes were renewed but replacement of the membranes did not solve the problem. To fnd the reasons and make a
comprehensive analysis, membrane autopsy was performed. Visual and physical inspection of the modules and some instrumental
analysis were conducted for membrane autopsy. Membranes were found severely fouled with organic and inorganic foulants. Main
foulant was iron which was deposited on surface. Te main reason was found to be the changing of aerator type of MBR. When
surface aerators were exchanged with bottom difusers which led to increasing of dissolved oxygen (DO) level of the basin, iron
particles were oxidized and they converted into particulate insoluble form. It was thought that probably this insoluble form of
the iron particles was the main cause of decreased membrane performance. Afer the diagnosis, a new pretreatment alternative
including a new iron antiscalant was suggested and system performance has been recovered.
1. Introduction
Membrane processes have many advantages due to their
modular designs, small footprints, and automated opera-
tions [1]. Tese advantages increased their usage within
very wide range of applications in water and wastewater
treatment. Despite this wide usage, membrane lifetime limits
the sustainability of the membrane processes. Widespread
use of membranes is still restricted because of membrane
fouling phenomena [2]. Membrane lifetime and performance
are afected by many factors such as selection of proper
process membrane material and operating parameters. Mem-
brane performance losses can be recognized by low efu-
ent rates, decreased rejection, high pressure drop between
inlet and outlet, and frequent cleaning requirement [3].
Optimum operation conditions decrease replacement period
and operating costs and increase membrane performance.
Another option to increase the lifetime of the membrane
is to apply pretreatment [4]. However, fouling is one of the
biggest problems in membrane area which negatively efects
membrane performance. Membrane fouling control is an
important subject and efective fouling control can be verifed
by membrane autopsy [5].
Renewal of membranes can be due to membrane clogging
or complete lifetime. Membrane autopsy may help to extend
membrane lifetime. Membrane autopsy can be thought of
as starting point for problem determination. It also gives
information about optimum operating conditions, chemi-
cal cleaning efectiveness, and the efects of infuent water
characteristics on membrane performance. According to the
studies, generally membranes encounter biofouling, metal
oxide fouling, oxidation, abrasion, and clay and mineral
Hindawi Publishing Corporation
e Scientific World Journal
Volume 2015, Article ID 850530, 8 pages
http://dx.doi.org/10.1155/2015/850530