American Journal of Biochemistry and Biotechnology 5 (4): 180-183, 2009
ISSN 1553-3468
© 2009 Science Publications
Corresponding Author: Syamsudin, Faculty of Pharmacy, Pancasila University, Jl., Srengseng Sawah, Jagakarsa,
South Jakarta, Indonesia
180
Chemical Composition of Propolis from Different Regions in
Java and their Cytotoxic Activity
1
Syamsudin,
2
Sudjaswadi Wiryowidagdo,
3
Partomuan Simanjuntak and
4
Wan Lelly Heffen
1
Department of Pharmacology,
2
Department of Biology of Pharmacy, Faculty of Pharmacy,
Pancasila University, Jl., Srengseng Sawah, Jagakarsa, South Jakarta, Indonesia
3
Department of Natural Product, Research Center for Biotechnology, Indonesian Institute of Sciences,
Jl. Raya Bogor km 46, West Java, Indonesia
4
Department of Research and Development, Dharmais Cancer Hospital, Jl. Letjen. S. Parman Kav 84-86,
West- Jakarta, Indonesia
Abstract: Problem statement: Propolis samples from tropical zones, such as Java (Indonesia) with its
vast biodiversity, have become a subject of increasing scientific and economic attention. The
association of the chemical composition of propolis from different geographic regions with cytotoxic
activities lead to the identification of active principles, a fundamental tool to achieve standardization of
this bee product. Approach: The purpose of this research was evaluate the quality of propolis
collected at different places in Java (Indonesia) based on cytotoxic activity. The ethanolic extracts of
propolis from different areas in Java were tested for cytotoxicity against tumor cell lines (T47D, MCF-
7, Hela, Myeloma and Vero) using MTT assay. Propolis samples were collected from Batang (Central
Java), Lawang (East Java) and Sukabumi (West Java). Results: The extract of propolis from Batang
showed the most potent activity of T47D and MCF-7 with IC
50
34.67±8.3 and 37.8±2.5 μg mL
-1
. The
extract of propolis from Sukabumi showed the most potent activity of Hela cell with IC
50
147.34±8.9.
However, all propolis extract did not show activity of myeloma and Vero cells. Conclusion: Ethanolics
extract of three propolis samples from Batang (Central Java), Lawang (East Java) and Sukabumi (West
Java) regions in Java were investigated using GC-MS. From 37 compounds identified, 7 among of
them were found for the first time in propolis. This indicated that the secondary metabolite extract of
propolis from Batang (Central Java) obtained in the study has antiproliferative activity of breast
carcinoma cells (T47D and MCF-7).
Key words: Propolis, Java, cytotoxicity activity, GC-MS, MTT assay
INTRODUCTION
Propolis is a resinous hive product collected by
honeybees (Apis mellifera, L.) from various plant
sources. Bees use it as a construction material, to
smooth internal walls of the hive and preserve it form
extreme moisture and drought condition. They also use
it to embalm dead invaders and in such way, prevent
the development and spread of microbial diseases.
Propolis is widely used in traditional medicine and is
reported to have of pharmacological activities. Besides
its traditional uses, it has recently gained popularity as a
food supplement in numerous countries, claimed to
improve health and prevent diseases
[2,3]
. Various
biological activities, such as anticancer, antioxidant,
antibiotic effects have been reported for propolis and its
components
[10]
.
The composition of the propolis depends on the
place and time of collection. As a consequence, more
than 160 components have been identified so far,
among which phenolic compounds, including
flavonoids, are major components
[4]
. Due to the
increasing interest in the characteristics of Indonesian
propolis, we undertook a study using samples collected
in different regions. We evaluated the quality of
propolis collected at different places in Java (Indonesia)
based on cytotoxic activity.
MATERIALS AND METHODS
Propolis: Propolis samples were collected from
different regions in Indonesia in April 2007 Sukabumi
(West Java), Batang (Central Java) and Lawang (East